Subjects -> CHEMISTRY (Total: 986 journals)
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    - INORGANIC CHEMISTRY (45 journals)
    - ORGANIC CHEMISTRY (47 journals)
    - PHYSICAL CHEMISTRY (71 journals)

ORGANIC CHEMISTRY (47 journals)

Showing 1 - 41 of 41 Journals sorted alphabetically
ACS Omega     Open Access   (Followers: 2)
Advances in Image and Video Processing     Open Access   (Followers: 18)
Advances in Physical Organic Chemistry     Full-text available via subscription   (Followers: 4)
Advances in Redox Research     Open Access   (Followers: 4)
American Journal of Organic Chemistry     Open Access   (Followers: 15)
Asian Journal of Organic Chemistry     Hybrid Journal   (Followers: 4)
Beilstein Journal of Organic Chemistry     Open Access   (Followers: 13)
Biochemia Medica     Open Access  
Current Organic Chemistry     Hybrid Journal   (Followers: 14)
Current Organic Synthesis     Hybrid Journal   (Followers: 12)
European Journal of Organic Chemistry     Hybrid Journal   (Followers: 59)
Herbal Medicine: Open Access     Open Access  
International Journal of Organic Chemistry     Open Access   (Followers: 9)
International Journal of Polymeric Materials     Hybrid Journal   (Followers: 6)
Journal of Bioactive and Compatible Polymers     Hybrid Journal   (Followers: 2)
Journal of Biomaterials Science, Polymer Edition     Hybrid Journal   (Followers: 9)
Journal of Organic Semiconductors     Open Access   (Followers: 6)
Journal of Peptide Science     Hybrid Journal   (Followers: 14)
Journal of Physical Organic Chemistry     Hybrid Journal   (Followers: 8)
Journal of Physiology and Biochemistry     Hybrid Journal   (Followers: 3)
Journal of Progressive Research in Chemistry     Open Access  
Journal of Proteins and Proteomics     Open Access   (Followers: 2)
Mini-Reviews in Organic Chemistry     Hybrid Journal   (Followers: 10)
Nigerian Journal of Chemical Research     Full-text available via subscription   (Followers: 1)
Open Journal of Organic Polymer Materials     Open Access   (Followers: 1)
Organic & Biomolecular Chemistry     Hybrid Journal   (Followers: 56)
Organic and Medicinal Chemistry Letters     Open Access   (Followers: 5)
Organic Chemistry : Current Research     Open Access   (Followers: 12)
Organic Chemistry Frontiers     Hybrid Journal   (Followers: 9)
Organic Chemistry International     Open Access   (Followers: 7)
Organic Geochemistry     Hybrid Journal   (Followers: 3)
Organic Letters     Hybrid Journal   (Followers: 92)
Organic Preparations and Procedures International: The New Journal for Organic Synthesis     Hybrid Journal   (Followers: 3)
Organic Process Research & Development     Hybrid Journal   (Followers: 32)
Progress in Organic Coatings     Hybrid Journal   (Followers: 7)
Reports in Organic Chemistry     Open Access   (Followers: 7)
Russian Journal of Organic Chemistry     Hybrid Journal   (Followers: 3)
Synthetic Communications: An International Journal for Rapid Communication of Synthetic Organic Chemistry     Hybrid Journal   (Followers: 31)
The Journal of Organic Chemistry     Hybrid Journal   (Followers: 135)
Vibrational Spectroscopy     Hybrid Journal   (Followers: 11)
World Journal of Organic Chemistry     Open Access   (Followers: 5)
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Organic Chemistry Frontiers
Journal Prestige (SJR): 2.155
Citation Impact (citeScore): 5
Number of Followers: 9  
 
  Hybrid Journal Hybrid journal (It can contain Open Access articles)
ISSN (Online) 2052-4129
Published by RSC Homepage  [49 journals]
  • Simple inorganic base promoted polycyclic construction using mucohalic
           acid as C3 synthon: Synthesis and AIE probe application of
           benzo[4,5]imidazo[1,2-a]pyridines

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01753E, Research ArticleKai Yang, Zhixi Chen, Yong-Jun Zhou, Qi Chen, Shi-Wei Yu, Shihe Luo, Zhaoyang Wang
      A transition metal-free and efficient synthesis of fused azapolycycles via multicomponent reaction has been developed from mucohalic acid as C3 synthon. The reaction promoted by simple inorganic base K2CO3 gives...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Generation of azaarene nitrile oxides from methyl azaarenes and t-BuONO
           enabling synthesis of furoxans and 1,2,4-oxadiazoles

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01872H, Research ArticleXiang-Jin Zhang, Jian-Kang Cao, Jun-Jie Ren, Lin Hong, Ru-Jin Liang, Kai-Yan Hao, Kai-Li Wei, Bao-Jing Mi, Yue Liu, Yan-Ping Zhu
      A high-efficiency strategy for the synthesis of furoxans and 1,2,4-oxadiazoles has been developed, utilizing tert-butyl nitrite (TBN) as nitrogen sources. Azaarene nitrile oxides as activated intermediates were generated in-situ via...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Correction: Electrochemically-mediated C–H functionalization of allenes
           and 1,3-dicarbonyl compounds to construct tetrasubstituted furans

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      Abstract: Org. Chem. Front., 2022, Advance Article

      DOI : 10.1039/D2QO90004A, CorrectionOpen Access Open Access Creative Commons Licence  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Mu-Xue He, Yan Yao, Chun-Zhi Ai, Zu-Yu Mo, Yu-Zheng Wu, Qi Zhou, Ying-Ming Pan, Hai-Tao Tang
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      DOI form of citation above.
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  • Novel pathway and seeded polymerizations of aggregates at the
           thermodynamic state for an amido-anthraquinone compound

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01848E, Research ArticleHouchen Wang, Mingyue Chen, Yuanyuan Zhu, Yu Li, Han Zhang, Tiesheng Shi
      Monomers ungergo supramolecular polymerizations via diversified pathways conferring pathway complexity; deciphering the complexity has been an intriguing and foundamental subject of studies. In this work, a functional anthraquinone molecule with...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Chiral Phosphoric Acid Catalyzed Regio- and Enantioselective Reactions of
           Functionalized Propargylic Alcohols

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01864G, Research ArticleChenxiao Qian, Meiwen Liu, Jianwei Sun, Pengfei Li
      Propargylic alcohols have been known as useful substrates in a wide range of asymmetric reactions. Particularly, the chiral phosphoric acids (CPAs) catalyzed reactions of functionalized propargylic alcohols opened a robust...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Aliphatic Sulfonyl Fluoride Synthesis via Reductive Decarboxylative
           Fluorosulfonylation of Aliphatic Carboxylic Acids NHPI Esters

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01655E, Research ArticleZhanhu Ma, Yongan Liu, Xiaoyu Ma, Xiaojun Hu, Yong Guo, Qing-Yun Chen, Chao Liu
      Based on radical sulfur dioxide insertion and fluorination strategy, we have developed an efficient method for aliphatic sulfonyl fluoride synthesis from abundant carboxylic acid, reductant, sulfur dioxide surrogate and electrophilic...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Regioselective Umpolung Addition of Dicyanobenzene to α,β-Unsaturated
           Alkenes Enabled by Electrochemical Reduction

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01852C, Research ArticleSheng Zhang, wenchao gao, Jianxue Shi, Jingjing Li, Fengyi Li, Yating Liang, Xuan Zhan, Man-Bo Li
      An umpolung addition of dicyanobenzene to α,β-unsaturated alkenes has been developed with an electroreductive strategy. This electrochemical protocol is well compatible with broad range of conventionally challenging substrates, including α,β-unsaturated...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Room temperature synthesis of perylene diimides facilitated by high amic
           acid solubility

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01723C, Research ArticleOpen Access Open Access Creative Commons Licence  This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Marcus C Kwakernaak, Marijn Koel, Peter J. L. van den Berg, E. M. Kelder, Wolter Jager
      A novel protocol for the synthesis of perylene diimides (PDIs), by reacting perylene dianhydride (PDA) with aliphatic amines is reported. Full conversions were obtained at temperatures between 20 and 60˚C,...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Origins of regio- and stereoselectivity in Cu-catalyzed alkyne
           difunctionalization with CO2 and organoboranes

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01788H, Research ArticleLingfei Hu, Han Gao, Yanlei Hu, Xiangying Lv, Yanbo Wu, Gang Lu
      The mechanism and origins of regio- and stereoselectivities of Cu-catalyzed alkyne difunctionalization with CO2 and trialkyl boranes were computationally investigated. The results show that the vicinal addition to alkyne is...
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  • How the electron-deficient Cp ligand facilitates Rh-catalyzed annulations
           with alkynes

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      Abstract: Org. Chem. Front., 2022, Advance Article

      DOI : 10.1039/D1QO01566D, Research ArticleHan Gao, Lingfei Hu, Yanlei Hu, Xiangying Lv, Yan-Bo Wu, Gang Lu
      The dominant factors for the CpX ligand effects (Cp* versus CpE) on the reactivity for alkyne insertion into cationic and neutral rhodacycles are identified based on energy decomposition analysis.
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  • Coordination-Assisted, Transition-Metal-Catalyzed Enantioselective
           Desymmetric C-H Functionalization

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01884A, Review ArticleXin Yu, Zhuo-Zhuo Zhang, Jun-Long Niu, Bing-Feng Shi
      Transition-metal-catalyzed asymmetric C-H functionalization has gradually emerged as a powerful tool for the creation of structural and chiral complexity in an atom- and step-economic fashion. The nature of this strategy...
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  • A Nickel/Organoboron Catalyzed Metallaphotoredox Platform for C(sp2)–P
           and C(sp2)–S Bond Construction

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01778K, Research ArticleYuan Zhu, Weisai Zu, Qing Tian, Zifeng Cao, Yu Wei, Liang Xu
      Herein, an organoboron photocatalyst, aminoquinolate diarylboron (AQDAB), is utilized collaboratively with nickel catalyst in metallaphotoredox catalyzed C(sp2)–P and C(sp2)–S cross-coupling reactions. This strategy effectively couples aryl halides with diarylphosphine oxides...
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  • Palladium-catalyzed decarbonylative methylation of aryl carboxylic acids

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01756J, Research ArticleBoya Feng, Guodong Zhang, Xu Feng, Yu Chen
      Described herein is a palladium-catalyzed decarbonylative methylation of aryl carboxylic acids using trimethylboroxine (TMB) as the methylating reagent. The Pd(OAc)2/XantPhos system is compatible with a wide range of carboxylic acids...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Acid-Catalyzed Ring-expansion of 4-(1-hydroxycyclobutyl)-1,2,3-triazoles

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01747K, Research ArticleMingchuan Xu, Lei Liu, Tao Wang, Han Luo, Meili Hou, Luan Du, Xiaolan Xin, Qixing Lu Lu, Baosheng Li
      We here reported a direct ring-opening/semipinacol rearrangement reaction of 4-(1-hydroxycyclobutyl)-1,2,3-triazole, in which N-acyl substituted 1,2,3-triazole was generated in situ and would trigger thermodynamically controlled electrocyclization ring-opening to afford rearrangement precursor...
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  • S-Triggered Schmidt-type Rearrangement of Vinyl Azides to Access
           N-Aryl-(trifluoromethylsulfinyl)acetamides

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01516H, Research ArticleZhenhua Liu, Tian Yu, Longhua Li, Wei Fu, Xingxing Gan, Huimin Chen, Wen Gao, Bo Tang
      A novel S-induced Schmidt-type rearrangement of vinyl azides with CF3SO2Na is reported, which is mediated by triphosgene (BTC) under mild reaction conditions. A wide range of N-arylated 2-(trifluoromethylsulfinyl)acetamieds, for the...
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  • Access to Enantioenriched Molecules with Diverse Fluorinated
           Tetrasubstituted Stereocenters Using Hydroxy as Kinetic Resolution
           Auxiliary Group

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01493E, Research ArticleXinqiang Fang, Syeda Tazeen Zehra, Shouang Lan, Hao Zhang, Jinggong Liu, Shuang Yang
      Developing a general method affording optically pure fully-substituted carbon molecules bearing various fluorinated groups is highly important but very challenging. Here we show that using secondary OH as the kinetic...
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  • Organocatalytic asymmetric synthesis of multifunctionalized
           α-carboline-spirooxindole hybrids that suppressed proliferation in
           colorectal cancer cells

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01785C, Research ArticleXiang-Hong He, Xue-Ju Fu, Gu Zhan, Nan Zhang, Xiang Li, Hong-Ping Zhu, Cheng Peng, Gu He, Bo Han
      Organocatalytic asymmetric [3 + 3] annulations of isatin-derived MBH carbonates and indolin-2-imines have been efficiently achieved. This appears to be the first enantioselective approach to use isatin-derived MBH carbonates as...
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  • Chemoselective Reduction of α,β-Unsaturated Ketones to Allylic Alcohols
           Under Catalyst-Free Conditions

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01754C, Research ArticleKaixia Jian, Bingnan Li, Shuxian Zhu, Qingqing Xuan, Qiuling Song
      Chemoselective reductions of α, β-unsaturated ketones to afford the corresponding allylic alcohols have always been challenging. Precious metals and ligands have always been employed in these transformations. Herein, we described...
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  • Visible light photocatalysis in synthesis of pharmaceutically relevant
           heterocyclic scaffolds

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01602D, Review ArticleVishal Srivastava, Pravin Kumar Singh, Shraddha Tivari, Praveen Pratap Singh
      Visible light and photoredox catalysis have emerged as a powerful and long-lasting tool for organic synthesis, demonstrating the importance of a variety of chemical bond formation methods. Natural products, physiologically...
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  • Iron-catalyzed multicomponent reaction of cycloketone oxime esters,
           alkenes, DABCO·(SO2)2 and trimethylsilyl azide

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01842F, Research ArticleJun Zhang, Junwei Wu, Xiaotong Chang, Peiqi Wang, Jiemin Xia, Jie Wu
      An iron-catalyzed four-component reaction of cycloketone oxime esters, alkenes, DABCO·(SO2)2 and trimethylsilyl azide (TMSN3) is described. This multicomponent radical transformation presents excellent regio- and chemo-selectivity, leading to a range of...
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  • Solvent-Controlled Regioselective Arylation of Indoles and Mechanistic
           Explorations

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01454D, Research ArticleShang-Dong Yang, Yuan Niu, Chaoxian Yan, Xin-Xin Yang, Pengbo Bai, Panpan Zhou
      The ability to manipulate the site selectivity in C–H bond functionalization reactions is an important goal in modern chemistry. Herein, we report a new reaction strategy for the regioselective arylation...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Visible Light Promoted Polyhalomethylation of Alkenes: Alkylation and
           Cyclization

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01662H, Research ArticleTong-Lin Wang, Bo-Sheng Zhang, Jingjiang Liu, Xiaojun Liu, Xi-Cun Wang, Zheng-Jun Quan
      We report a visible light promoted carbochloromethylation of 2-bromomethyl acrylate and N-arylmethacrylamide, and a series of trihalomethyl substituted allylic acid esters and indolone derivatives were synthesized. The reaction used common...
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  • RhIII-catalyzed heteroarylation of N-2,6-difluorophenyl arylamides with
           heteroaryl boronate esters

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01868J, Research ArticleJia-Xue Wu, Qing-Xia Yao, Wen-zeng Duan, DaCheng Li, Xianqiang Huang, Jian-Min Dou, Huaiwei Wang
      Herein, an efficient strategy to aryl-heteroaryl formation via RhIII-catalyzed ortho-C(sp2)−H heteroarylation of (hetero)arenes with heterocyclic boronates using a readily removable N-2,6-difluorophenyl arylamides directing group has been disclosed. A variety of...
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  • Regio- and stereo-selective olefinic C-H functionalization of aryl alkenes
           in ethanol

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01676H, Research ArticleJian Zhang, Shuqi Jin, Cong Shen, Kejie Xu, Guofu Zhong, Yuhang Zhu, Lixia Xu, Shuxin Luo, Liangjun Zhong
      We report on N,N-bidentate-chelation-assisted α- and β-olefinic C-H alkenylation of aryl alkenes in ethanol to afford aryl dienes/trienes with excellent regio- and stereo-selectivities. The reaction of 2-alkenyl benzylamine and benzoic...
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  • Oxidative thiocyanation of allylic alcohols: an easy access to allylic
           thiocyanate within K2S2O8 and NH4SCN

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01710A, Research ArticleKeyuan Zhang, Tianbing Liang, Yulong Wang, Chonglong He, Mingyou Hu, Xin-Huan Duan, Le Liu
      A practical method for the synthesis of allylic thioacyanate from allylic alcohol was disclosed employing K2S2O8 as the oxidant and NH4SCN as the thiocyanate source. Without introducing a leaving group...
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  • Iron-Catalyzed decarboxylative and oxidative decarbonylative
           cross-coupling: A new strategy for the synthesis of monofluoroalkenes

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01567B, Research ArticleXiao-Yu Lu, Meng-Yuan Ge, Ting-Hua Tao, Xiao-Mei Sun, Meng-Ting Gao, Shu-Ting Bao, Qi-Le Liu, Ze-Jie Xia, Jing Xia
      Herein, an iron(II)-catalyzed decarboxylative and oxidative decarbonylative cross-coupling of α-fluoroacrylic acids with aliphatic aldehydes is presented. This methodology provided a novel and practical strategy for the construction of the monofluoroalkenes...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • DFT study on ruthenium-catalyzed decarbonylative annulation of an alkyne
           with six-membered hydroxychromone via C−H/C−C activation

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01786A, Research ArticleHong-Jing Long, Lei Zhang, Bing Lian, De-Cai Fang
      We report a density functional theory study on ruthenium-catalyzed decarbonylative annulation of an alkyne with six-membered hydroxychromone via C−H/C−C Activation. The plausible catalytic cycles involve O−H deprotonation, C−H activation, alkyne...
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  • post-Spin Crossing Dynamics Determine the Regioselectivity in Open-shell
           Singlet Biradical Recombination

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01757H, Research ArticleMin Zhu, Chao Zheng
      Radical recombination is among the fastest reactions in organic chemistry. Achieving high level of selectivities in this type of reactions is rather challenging. In a recent report on visible-light-induced dearomative...
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  • Pyrylium Salts Acting as Both Energy Transfer and Electron Transfer
           Photocatalysts for E→Z Isomerization of Activated Alkenes and
           Cyclization of Cinnamic or Biaryl Carboxylic Acids

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01623G, Research ArticleLei Bao, Jin-Tang Cheng, Zhi-Xiang Wang, Xiang-Yu Chen
      2,4,6-Triarylpyrylium salts are stable, easily available and cheap. However, only their elec-tron transfer oxidation ability was explored. We herein report that they could perform both energy transfer and electron transfer...
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  • Photoinduced C-H monofluoroalkenylation with gem-difluoroalkenes through
           hydrogen atom transfer in batch and flow

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01689J, Research ArticleChen-Lin Cao, Guang-Xu Zhang, Fei Xue, Hong-Ping Deng
      Direct monofluoroalkenylation of C-H bonds are straightforward approaches for accessing multisubstituted monofluoroalkenes. However, general methods for the monofluoroalkenylation of C(sp3)-H bonds remain challenges. Here we report the development of a...
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  • Synthesis of Acridinones via Palladium-Catalyzed Reductive Annulation of
           2-Nitrobenzaldehydes and Resorcinols

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01693H, Research ArticleRong Xie, Wenhui Mao, Huanhuan Jia, Guangpeng Lu, Jialu Sun, Huanfeng Jiang, He Zhao, Min Zhang
      Catalytic conversion of biomass-derived feedstocks into functional molecules is of significance to synthetic organic chemistry. Herein, through a palladium-catalyzed reductive annulation reaction of resorcinols and 2-nitrobenzaldehydes, we present a new...
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  • Cu(II)-Catalyzed C2-Site Functionalization of p-Aminophenols: An Approach
           of Selective Cross-Dehydrogenative Aminations

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01675J, Research ArticleXin Zhao, Fang Yang, Lin-Lin Wang, Jing Guo, Yu-Qin Xu, Zi-Sheng Chen, Kegong Ji
      The site selective cross dehydrogenative aminations from precursors without preactivated C-H and N-H bonds has been challenging. Herein, a copper-catalyzed C2-site selective amination of p-aminophenol derivatives with arylamines had been...
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  • Palladium-Catalyzed Tandem Heck/Carbonylation/Aminocarbonylation En Route
           to Chiral Het-erocyclic α-Ketoamides

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01680F, Research ArticleHuaanzi Hu, Ting Yu, Sidi Cheng, Jing Li, Chunfang Gan, Shuang Luo, Qiang Zhu
      An unprecedented tandem carbonylation/aminocarbonylation triggered by palladium-catalyzed enantioselective Heck-type exocyclopalladation delivering chiral heterocyclic α-ketoamides has been developed. The uncommon double CO insertion into the σ-alkylpalladium intermediate takes place selectively under...
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  • Rh-Catalyzed Diastereoselective Addition of Arylboronic Acids to α-Keto
           N-tert-Butanesulfinyl Aldimines: Synthesis of α-Amino Ketones

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01721G, Research ArticleCece Wang, Lu Zhou, Jian Qiu, Kai Yang, Qiuling Song
      Herein we present a diastereoselective addition of arylboronic acids to α-keto N-tert-butanesulfinyl aldimines catalyzed by Rh(I) catalyst. This reaction provides a practical method to deliver valuable chiral α-amino ketones with...
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  • Isotopic Labelling Experiments and Enzymatic Preparation of Iso-Casbenes
           with Casbene Synthase from Ricinus communis

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01707A, Research ArticleHeng Li, Jeroen Dickschat
      Isotopic labelling experiments gave insights into the enzyme mechanism of casbene synthase from Ricinus communis, showing a clear stereochemical course for the cyclisation reaction, in agreement with the reported absolute...
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  • Euphorstranoids A and B, Two Highly Rearranged Ingenane Diterpenoids from
           Euphorbia stracheyi: Structural Elucidation, Chemical Transformation, and
           Lipid-Lowering Activity

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01705E, Research ArticleFang-Yu Yuan, Yue-Hua Pan, Ai-Ping Yin, Wei Li, Dong Huang, Xue Long Yan, Shu-Qi Wu, Gui-Hua Tang, Rong Pu, Sheng Yin
      Euphorstranoids A (1) and B (2), two highly rearranged ingenane diterpenoids with an unusual 5/6/7/3 carbon ring system, were isolated from Euphorbia stracheyi. Their structures were determined by a combination...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Water-promoted regio-selective trifluoromethylation of vinyl conjugated
           diazoacetates

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      Abstract: Org. Chem. Front., 2022, 9,204-209

      DOI : 10.1039/D1QO01654G, Research ArticleXinxin Han, Xin Liu, Yueyun Bao, Hunahuan Song, Yu-Rou Zhao, Xiaoying Wang, Junjie Zhang, Le Liu, Xin-Hua Duan, Jinbo Hu, Mingyou Hu
      An efficient trifluoromethylation reaction of vinyldiazoacetates under mild reaction conditions was depicted.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Efficient enantioselective synthesis of CF2H-containing
           dispiro[benzo[b]thiophene-oxindole-pyrrolidine]s via organocatalytic
           cycloaddition

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      Abstract: Org. Chem. Front., 2022, 9,210-215

      DOI : 10.1039/D1QO01392K, Research ArticleYabo Deng, Yongzhen Li, Yalan Wang, Shuo Sun, Sichao Ma, Pengfei Jia, Wenguang Li, Kairong Wang, Wenjin Yan
      A novel kind of CF2H-containing dispiro[benzo[b]thiophene-oxindole-pyrrolidine] has been achieved via an organocatalyzed 1,3-dipole reaction.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • A multifaceted approach towards understanding the peculiar behavior of
           (α)-hydroxyiminophosphonates

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      Abstract: Org. Chem. Front., 2022, 9,173-182

      DOI : 10.1039/D1QO01564H, Research ArticleThomas Toupy, Christopher Kune, Kristof Van Hecke, Loïc Quinton, Jean-Christophe M. Monbaliu
      A unique multifaceted approach involving the interplay of NMR, XRD, LC, DFT and MS/IM-MS techniques toward the understanding of the peculiar isomer-selective reduction of (α)-hydroxyiminophosphonates into (α)-hydroxyaminophosphonate derivatives.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Palladium-catalysed stereoselective [3 + 2] annulation of vinylethylene
           carbonates and tryptanthrin-based ketones

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      Abstract: Org. Chem. Front., 2022, 9,197-203

      DOI : 10.1039/D1QO01543E, Research ArticleYang Fan, Qing-Zhu Li, Jun-Long Li, Bin Zhang, Zhen Dai, Ke Xie, Rong Zeng, Liang Zou, Xiang Zhang
      The first example of palladium-catalysed [3 + 2] annulation of VECs and ketones has been developed, allowing the efficient synthesis of indoloquinazolinones in generally excellent yields with good stereoselectivity.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • The first N-ligand assisted Pd catalyzed asymmetric synthesis of
           3-arylsuccinimides as novel antifungal leads

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      Abstract: Org. Chem. Front., 2022, 9,183-189

      DOI : 10.1039/D1QO01510A, Research ArticleJixing Lai, Juan Yang, Chen Yang, René Csuk, Baoan Song, Shengkun Li
      The first palladium/chiral nitrogenous ligand-catalyzed enantioselective addition of aryl boronic acids to various maleimides was reported.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Fissisternoids A and B, two 2′,5′-quinodihydrochalcone-based
           meroterpenoid enantiomers with unusual carbon skeletons from Fissistigma
           bracteolatum

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, 9,190-196

      DOI : 10.1039/D1QO01404H, Research ArticleGui-Min Xue, Chen-Guang Zhao, Jin-Feng Xue, Hui Chen, Zhen-Zhu Zhao, Ying-Ying Si, Kun Du, Yan-Le Zhi, Wei-Sheng Feng
      Compound 1 represents an unprecedented meroterpenoid featuring a unique tricyclo [3,3,1,01′,5′] decane central framework and 2 possesses a rare 6/6/5/4 tetracyclic carbon skeleton were isolated from Fissistigma bracteolatum.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Gold self-relay catalysis for accessing functionalized cyclopentenones
           bearing an all-carbon quaternary stereocenter

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      Abstract: Org. Chem. Front., 2022, 9,140-146

      DOI : 10.1039/D1QO01313K, Research ArticleFan-Tao Meng, Jing-Long Chen, Xiao-Yan Qin, Tian-Shu Zhang, Shu-Jiang Tu, Bo Jiang, Wen-Juan Hao
      A new gold(I) self-relay catalysis consisting of a 3,3-rearrangement, Nazarov cyclization and Michael addition cascade of 1,3-enyne acetates with aurones and their derived azadienes is reported, producing functionalized cyclopentenones.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • One-pot enantioselective construction of 3,4-dihydro-2H-1,4-oxazines over
           Ru/Au relay catalysis and its mechanistic serendipity

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      Abstract: Org. Chem. Front., 2022, 9,102-108

      DOI : 10.1039/D1QO01482J, Research ArticleDongfeng Yang, Chengyi Wang, Yu Wang, Guohua Liu, Tanyu Cheng, Rui Liu
      One-pot enantioselective construction of 3,4-dihydro-2H-1,4-oxazines have been developed through the transfer hydrogenation/cyclization enantio-relay process using Ru and Au bimetallic catalysts.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Key role of a π–π complex in diaryl cross-coupling between
           aryldiazonium salts and arylboronic acids using photosensitizer-free
           gold/photoredox catalysis

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, 9,147-155

      DOI : 10.1039/D1QO01464A, Research ArticleYanhong Liu, Rongxiu Zhu, Chengbu Liu, Dongju Zhang
      In a new mechanism for photosensitizer-free visible-light-mediated gold-catalyzed cross-coupling, the π–π complex between aryldiazonium salts and arylboronic acids acts as a photoinitiator.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • A mechanistic study on the regioselective Ni-catalyzed
           methylation–alkenylation of alkyne with AlMe3 and allylic alcohol

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      Abstract: Org. Chem. Front., 2022, 9,163-172

      DOI : 10.1039/D1QO01580J, Research ArticleJiao Liu, Deguang Liu, Wan Nie, Haizhu Yu, Jing Shi
      The recently reported Ni-catalyzed methylation–allylation of alkynes with allylic alcohols and AlMe3 reagents delivers valuable tetrasubstituted alkene units in a highly regioselective fashion.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Transition-metal-free hydroamination/defluorination/cyclization of
           perfluoroalkyl alkynes with amidines

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, 9,109-116

      DOI : 10.1039/D1QO01439K, Research ArticleLi-Wen Sun, Zi-Lun Yu, Xin-Long Luo, Mengtao Ma, Zhi-Liang Shen, Xue-Qiang Chu
      An efficient defluorinative cyclization strategy for the construction of perfluoroalkyl-substituted pyrimidines by using perfluoroalkyl alkynes and amidines as substrates was developed.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Palladium-catalyzed direct construction of oxazoline-containing polycyclic
           scaffolds via tandem addition/cyclization of nitriles and arylboronic
           acids

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      Abstract: Org. Chem. Front., 2022, 9,123-128

      DOI : 10.1039/D1QO01260F, Research ArticleShu-Qiang Cui, Na Cheng, Qian-Qian Ma, Zhong-Lin Wei, Wei-Wei Liao
      An efficient construction of oxazoline-containing polycyclic scaffolds through a Pd-catalyzed addition/cyclization of (hetero)arene tethered O-acyl cyanohydrin units and arylboronic acids is described.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Gold-catalysed synthesis of phosphonate-substituted oxetan-3-ones – an
           easy access to highly strained HWE reagents

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      Abstract: Org. Chem. Front., 2022, 9,117-122

      DOI : 10.1039/D1QO01214B, Research ArticleShaista Tahir, Jonas F. Wunsch, Matthias Rudolph, Frank Rominger, A. Stephen K. Hashmi
      Gold-catalysed reaction of alkynyl phosphonates to attain alkenyl substituted oxetan-3-ones via subsequent HWE reaction.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • In situ phosphonium-containing Lewis base-catalyzed 1,6-cyanation
           reaction: a facile way to obtain α-diaryl and α-triaryl acetonitriles

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      Abstract: Org. Chem. Front., 2022, 9,156-162

      DOI : 10.1039/D1QO01501J, Research ArticleJian-Ping Tan, Yuan Chen, Xiaoyu Ren, Yumeng Guo, Bing Yi, Hongkui Zhang, Guowei Gao, Tianli Wang
      A in situ phosphonium-containing catalyst and its successful application in promoting remote 1,6-cyanation reaction of p-QMs and fuchsones have been disclosed, providing a facile and direct access to both α-diaryl and α-triaryl acetonitriles.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • A combined experimental and computational study of NHC-catalyzed
           allylation of allenoate with MBH esters: new regiospecific and
           stereoselective access to 1,5-enyne

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, 9,51-57

      DOI : 10.1039/D1QO01083B, Research ArticleFang Sun, Fangfang Lu, Xue Song, Wenchao Wu, Kai Zhang, Chenxia Yu, Tuanjie Li, Donghui Wei, Changsheng Yao
      An NHC-catalyzed regiospecific allylation of α-substituted allenoates with MBH carbonates derived from aryl aldehyde furnished highly functionalized 1,5-enynes.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Enantioselective total syntheses of marine natural products
           (+)-cylindricines C, D, E and their diastereomers

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, 9,58-63

      DOI : 10.1039/D1QO01408K, Research ArticleYing-Hong Huang, Zhan-Jiang Liu, Pei-Qiang Huang
      On the basis of the amide strategy, we have achieved the concise enantioselective total synthesis of (+)-cylindricines D, C, and E, and their 2-epimers in seven, eight, and nine steps, respectively.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • “The red cage”: implementation of pH-responsiveness within a
           macrobicyclic pyridinium-based molecular host

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      Abstract: Org. Chem. Front., 2022, 9,81-87

      DOI : 10.1039/D1QO01331A, Research ArticlePablo Cortón, Hongye Wang, Iago Neira, Arturo Blanco-Gómez, Elena Pazos, Carlos Peinador, Hao Li, Marcos D. García
      The “red cage”, a new pyridinium-based macrobicyclic host, has been found to complex model aromatic substrates in aqueous media in a pH-responsive fashion.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Three decades of unveiling the complex chemistry of C-nitroso species with
           computational chemistry

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      Abstract: Org. Chem. Front., 2022, 9,223-264

      DOI : 10.1039/D1QO01415C, Review ArticlePauline Bianchi, Jean-Christophe M. Monbaliu
      This review revisits the complex reactivity of C-nitroso derivatives through the synergistic combination of computational and synthetic organic chemistry, with an emphasis on the rationalization of mechanisms and selectivities.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Insight into the mechanism of the arylation of arenes via norbornene relay
           palladation through meta- to para-selectivity

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      Abstract: Org. Chem. Front., 2022, 9,129-139

      DOI : 10.1039/D1QO01500A, Research ArticleShengnan Liu, Qiong Wang, Fang Huang, Wenjuan Wang, Chong Yang, Jianbiao Liu, Dezhan Chen
      A theoretical insight was shown into the origin of site-selectivity in the arylation of arenes by a norbornene relay palladation through meta- to para-selectivity.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • DBU-catalyzed dearomative annulation of 2-pyridylacetates with
           α,β-unsaturated pyrazolamides for the synthesis of multisubstituted
           2,3-dihydro-4H-quinolizin-4-ones

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, 9,88-94

      DOI : 10.1039/D1QO01414E, Research ArticleYao-Bin Shen, Jian-Qiang Zhao, Zhen-Hua Wang, Yong You, Ming-Qiang Zhou, Wei-Cheng Yuan
      DBU-catalyzed dearomative [3 + 3] annulation of 2-pyridylacetates and α,β-unsaturated pyrazolamides for the synthesis of multisubstituted 2,3-dihydro-4H-quinolizin-4-ones was developed.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Alkyl-modified nucleobases with 6/5/7/5 ring systems from the insect
           Cyclopelta parva

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      Abstract: Org. Chem. Front., 2022, 9,75-80

      DOI : 10.1039/D1QO01603B, Research ArticleYong-Ming Yan, Heng Chen, Wen-Long Chen, Dai-Wei Wang, Li Liao, Qing Lu, Yong-Xian Cheng
      (±)-Cyclopeltains A and B (1 and 2), two pairs of unusual alkylated adenine derivatives, were isolated from the insect Cyclopelta parva and structurally characterized.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Electrochemical synthesis of functionalized gem-difluoroalkenes with
           diverse alkyl sources via a defluorinative alkylation process

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, 9,95-101

      DOI : 10.1039/D1QO01460A, Research ArticleHaoxiang Zhang, Mengze Liang, Xiao Zhang, Meng-Ke He, Chao Yang, Lin Guo, Wujiong Xia
      An electrochemical defluorinative alkylation of α-trifluoromethyl alkenes is described. This reaction enables the preparation of functionalized gem-difluoroalkenes with diverse alkyl sources including organohalides, NHP esters, and Katritzky salts.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Molecular rotor based on an oxidized resorcinarene

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      Abstract: Org. Chem. Front., 2022, 9,39-50

      DOI : 10.1039/D1QO01479J, Research ArticleDaniel T. Payne, Jan Labuta, Zdeněk Futera, Václav Březina, Lenka Hanyková, Mandeep K. Chahal, Jonathan P. Hill
      Rate of rotation of substituents in a molecular single stator-double rotor based on an oxidized resorcinarene with unsaturated hemiquinonoid groups at its meso positions (i.e., a fuchsonarene) has been controlled according to solvent polarity and acidity.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Sequence-sorted redox-switchable hetero[3]rotaxanes

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, 9,64-74

      DOI : 10.1039/D1QO01553B, Research ArticleOpen Access Open Access Creative Commons Licence  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Marius Gaedke, Henrik Hupatz, Felix Witte, Susanne M. Rupf, Clara Douglas, Hendrik V. Schröder, Lukas Fischer, Moritz Malischewski, Beate Paulus, Christoph A. Schalley
      Programming the sequence of functional units in redox-switchable hetero[3]rotaxanes is achieved by integrative self-sorting for a library of five crown ethers.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • K2S2O8-mediated acylarylation of unactivated alkenes via acyl radical
           addition/C–H annulation cascade of N-allyl-indoles with silver
           cocatalysis

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, 9,32-38

      DOI : 10.1039/D1QO01069G, Research ArticleJitan Zhang, Manyi Wu, Hu Ju, Haitao Yang, Baiyang Qian, Ke Ding, Jiaping Wu, Meihua Xie
      A silver-catalyzed, K2S2O8-mediated protocol to access the regioselective acylarylation of unactivated alkenes was reported.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Visible light-promoted aerobic oxidative cleavage and cyclization of
           olefins to access 3-hydroxy-isoindolinones

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      Abstract: Org. Chem. Front., 2022, 9,25-31

      DOI : 10.1039/D1QO01087E, Research ArticleTao Ma, Jiawei Hua, Mixue Bian, Hong Qin, Xinxin Lin, Xiaobing Yang, Chengkou Liu, Zhao Yang, Zheng Fang, Kai Guo
      An environmentally friendly synthetic approach is described from 2-vinylbenzamide to 3-hydroxy-isoindolinones through visible light-promoted transformations via iron/disulfide catalysis and molecular oxygen oxidation.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Electrochemical oxidative cyclization of alkenes, boronic acids, and
           dichalcogenides to access chalcogenated boronic esters and 1,3-diols

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      Abstract: Org. Chem. Front., 2022, 9,12-18

      DOI : 10.1039/D1QO01175H, Research ArticleChangfeng Huang, Jijing Hu, Guangxian Chen, Minjian Wu, Hua Cao, Xiang Liu
      A sustainable, environmentally benign electrochemical oxidative three-component cyclization of allylic alcohols, boronic acids, and dichalcogenides under metal-free and oxidant-free conditions has been developed.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Diastereodivergent synthesis of fully disubstituted
           spiro[indoline-3,2′-pyrrolidin]-2-ones via tuneable Lewis base/Brønsted
           base-promoted (3 + 2) cycloadditions

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, 9,19-24

      DOI : 10.1039/D1QO01124C, Research ArticleKe Li, Zhipeng Zhang, Jiahui Zhu, Yuxin Wang, Jing Zhao, Er-Qing Li, Zheng Duan
      We have developed unique base-promoted diastereoselective (3 + 2) cycloadditions. A diastereodivergent synthesis of fully disubstituted spiro[indoline-3,2′-pyrrolidin]-2-ones was realized by tuning a Lewis base/Brønsted base.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Recent advances in catalytic enantioselective direct C–H bond
           functionalization of electron-deficient N-containing heteroarenes

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      Abstract: Org. Chem. Front., 2022, 9,265-280

      DOI : 10.1039/D1QO01223A, Review ArticleXiao-Lan Liu, Luo-Bin Jiang, Mu-Peng Luo, Zhi Ren, Shou-Guo Wang
      Catalytic enantioselective direct C–H bond functionalization of electron-deficient N-containing heteroarenes represents one of the most straightforward and powerful protocols to construct diverse enantioenriched highly functionalized N-heteroarenes.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Construction of Axially Chiral Styrene-Type Allylamines via Chiral
           Phosphoric Acid-Catalyzed Asymmetric Reductive Amination

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01672E, Research ArticleYou-Dong Shao, Jin-Shuo Feng, Dan-Dan Han, Kang-Hui Pan, Ling Zhang, Yi-Fan Wang, Zhong-Hui Ma, Pei-Ru Wang, Mingjing Yin, Dao-Juan Cheng
      The first enantioselective synthesis of axially chiral styrene-type allylamines was achieved through chiral phosphoric acid mediated atroposelective reductive amination of 1-enal substituted 2-naphthols. This protocol features a broad substrate scope,...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Palladium-catalyzed stereoselective trifluoromethylated allylic alkylation
           of 3-substituted oxindoles

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01597D, Research ArticleDong Li, Shuaibo Zhang, Bangzhong Wang, Wuding Sun, Jinfeng Zhao, Jingping Qu, Yuhan Zhou
      An efficient catalytic methodology for trifluoromethylated allylic alkylation of 3-substituted oxindoles using α-(trifluoromethyl)alkenyl acetates as trifluoromethyl-containing allylic alkylation partner is described. The reaction proceeds smoothly with the incorporation of Pd(OAc)2...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • RhodiumIII-Catalyzed Successive Csp2‒H and Csp2‒Csp2 Bond Activation
           of Aryl Oximes: Synthetic and Mechanistic Studies

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01669E, Research ArticleGuo-Jun Deng, Cheng Li, Fuhong Xiao, Huawen Huang, Bin Zhao
      Merging selective C–H cleavage with C–C cleavage in a tandem reaction has been a practical strategy that permits skeletal diversification from simple raw materials. Herein, we describe a rhodiumIII-catalyzed redox-neutral...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • 1D alignment of proteins and other nanoparticles by using reversible
           covalent bonds on cyclic peptide nanotubes

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01349A, Research ArticleJuan R Granja, Javier Montenegro, Iria Louzao, Ivan Gallego, Juan Manuel Priegue
      Self-assembling cyclic peptide nanotubes are supramolecular structures whose diameter and external surface properties are precisely controlled. In this communication we describe a general strategy to align different molecules on top...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Synthesis of Functionalized 3,2′-Pyrrolidinyl Spirooxindoles via Domino
           1,6-Addition/Annulation Reactions of para-Quinone Methides and
           3-Chlorooxindoles

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01605A, Research ArticleYang Wang, Xiaochen Tian, Yongxing Zhang, Weiwu Ren
      A highly efficient base-mediated diastereoselective [4+1] cycloaddition of ortho-tosylaminophenyl-substituted p-QMs with 3-chlorooxindoles has been developed to afford 3,2’-pyrrolidinyl spirooxindoles in high yields with high diastereoselectivity through domino 1,6-addition/cyclization sequence. This...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Selective 1,4-Arylsulfonation of 1,3-Enynes via Photoredox/Nickel Dual
           Catalysis

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01653A, Research ArticleChao Li, Duo-Duo Hu, Ruoxing Jin, Bing-Bing Wu, Cheng-Yu Wang, Zhuofeng Ke, Xi-Sheng Wang
      A photoredox/nickel-catalyzed selective 1,4-arylsulfonation of 1,3-enynes to access structurally diverse sulfone-containing allenes has been established. This radical cascade transformation featured with easy manipulation, mild conditions, low catalyst loading, broad substrate...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Electrochemically-mediated C-H functionalization of allenes and
           1,3-dicarbonyl compounds to construct tetrasubstituted furans

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01458G, Research ArticleMu-Xue He, Yan Yao, Chun-Zhi Ai, Zu-yu Mo, Yu-Zheng Wu, Qi Zhou, Ying-Ming Pan, Hai-Tao Tang
      C-H functionalization of allenes is an available strategy to construct heterocyclic compounds. Herein we propose a sus-tainable electrocatalytic C-H activation for the synthesis of novel highly functionalized tetrasubstituted furans, which...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Synthesis of 2-trifluoromethyl chromenes via double carbonyl-ene reaction

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01766G, Research ArticleShouxiong Chen, Hui Wang, Qi Lin, Zhiqiang Weng
      A new protocol for the synthesis of diversely substituted 2-trifluoromethyl chromenes from the cyclization reaction of o-isopropenylphenols with trifluoroacetic anhydride has been developed, which proceeds via sequential trifluoroacetylation and double...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Silver-catalyzed [3+3]-annulation cascade of alkynyl alcohols and
           α,β-unsaturated ketones for the regioselective assembly of chromanes

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01643A, Research ArticleAshwini Kadaji Nakate, Sagar Sudam Thorat, Shailja Jain, Rama Krishna Gamidi, Kumar Vanka, Ravindar Kontham
      An unprecedented Ag(I)-catalyzed [3+3]-annulation of alkynyl alcohols (5-hexyn-1-ols) and α,β-unsaturated ketones is reported to construct simple to complex chromanes. This transformation begins with hydroalkoxylation of alkynol through C-C triple bond...
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  • Recent developments in the asymmetric synthesis and functionalization of
           symmetrical and unsymmetrical gem-diborylalkanes

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      Abstract: Org. Chem. Front., 2022, Advance Article

      DOI : 10.1039/D1QO01300A, Review ArticleSwagata Paul, Kanak Kanti Das, Debasis Aich, Samir Manna, Santanu Panda
      gem-Diborylalkanes are an important class of organoboron compounds as they function as a key building block in organic synthesis. This review summarizes recent developments of the enantioselective synthesis of gem-diborylalkanes and application in asymmetric synthesis.
      To cite this article before page numbers are assigned, use the
      DOI form of citation above.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Carbene-Enabled Ether Activation Through the Formation of Oxonium: A
           Theoretical View

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01730F, Research ArticleYa-Nan Wang, Xinghua Wang, Shi-Jun Li, Yu Lan
      Here, we report a theoretical investigation of the reactivity and chemoselectivity of carbene-enabled ether activation. The mechanism obtained from DFT calculations revealed that the final products were dependent on the...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Organocatalytic Difluorobenzylation of 1,2-Diketones via Mild Cleavage of
           Carbon−Carbon Bonds

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01645H, Research ArticleYong Zhang, Guo-Wei Lai, Long-Jun Nie, Qifang He, Mei-Juan Lin, Rong Chi, Dong-Liang Lu, Xiaolin Fan
      α-aryl-α,α-Difluoroacetophenones (DFAPs) are developed as a new type of difluorobenzylation reagents that can be facilely prepared from readily available and cheap starting materials. In-situ carbon-carbon bond cleavage of electron-deficient DFAPs...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Recent Advances of Transition-Metal-Free Trifluoromethylation with
           Togni’s Reagents

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01504D, Review ArticleJin-Yang Chen, Jing Huang , Kai Sun, Wei-Min He
      Developments in transition-metal-free trifluoromethylation have attracted broad interests driven by the increasing importance of CF3-containing compounds. Among diverse trifluoromethylation reagents, Togni’s reagents displayed exceptional reactivities, and abundant meaningful organic transformations...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • One-pot synthesis of natural-product inspired spiroindolines with
           anti-cancer activities

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01694F, Research ArticleShiqiang Li, Wei Yan, Liu-Jun He, Ming Zhang, Dianyong Tang, Hong-yu Li, Zhongzhu Chen, Zhigang Xu
      A post-Ugi/diastereoselective cascade reaction was developed to construct naturally existing spiroindolines via a facile and metal-free one-pot protocol. During the construction, a new C-C bond was formed through a selective...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Ni(ǁ)-catalyzed Reductive Cross-coupling Reaction of Oxalates and
           Thiosulfonates/Selenosulfonates

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01614H, Research ArticleYing Chen, Fei Wang, Bo-Xi Liu, Weidong Rao, Shun-Yi Wang
      A Ni(ǁ)-catalyzed reductive cross-coupling reaction of oxalates and thiosulfonates/selenosulfonates to synthesize benzylic sulfides/selenides under mild conditions is developed. The oxalates prepared from the corresponding alcohols are used as carbon radical...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Total Syntheses of Seven Stemoamide-Type Stemona Alkaloids

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01578H, Research ArticleTao Shi, Fei Cao, Jin hong Chen, Xiao-Dong Wang, Gaofeng Yin, Huihong Wang, Zhen Wang
      Six Stemona alkaloids were synthesized racemically by using stemoamide, obtained via cascade cyclization or our reported transannular cyclization of parvistemoamide, as the common intermediate. Thioamides facilitated the separation of isosaxorumamide...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Electrochemical Radical C(sp3)-H Arylation of Xanthenes with Electron-Rich
           Arenes

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01714D, Research ArticleBin Wei, Jing-Hao Qin, Yong-Zheng Yang, Ye-Xiang Xie, Xuan-Hui Ouyang, Ren-Jie Song
      C(sp3)-H arylation has recently emerged as a powerful straegy for complex organic molecules synthesis through a new carbon-carbon bond formation. We herein describe an efficient electrochemical C(sp3)-H arylation of xanthenes...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • The extended Corey-Chaykovsky reactions: transformation of
           2-hydroxychalcones to benzannulated 2,8-dioxabicyclo[3.2.1]octanes and
           2,3-dihydrobenzofurans

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01646F, Research ArticleAlexander A. Fadeev, Anton S. Makarov, Olga Alexandrovna Ivanova, Maxim G. Uchuskin, Igor V. Trushkov
      We report the divergent synthesis of benzannulated 2,8-dioxabicyclo[3.2.1]octanes and 2,3-dihydrobenzofurans using the concept of the extended Corey-Chaykovsky reactions. With this concept, 2-hydroxychalcones were treated with the Corey ylide providing highly...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Silver-catalyzed stereoselective C-4 arylthiodifluoromethylation of
           coumarin-3-carboxylic acids via a double decarboxylative strategy

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01609A, Research ArticleZhiwei Chen, Jie Sun, Zhiwei Ke, Xiaoxiao Huang, Ziwei Li
      A facile silver-catalyzed dual decarboxylation of arylthio-difluoroacetic acid with coumarin-3-carboxylic acids/chromone-3-carboxylic acids was developed. This method provided a unique way to synthesize a series of C-4 arylthiodifluoromethylated 3,4-dihydrcoumarins/C-2 arylthiodifluoromethylated chromanones...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • O-BODIPYs as fluorescent labels for sugars: glucose, xylose and ribose

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01418H, Research ArticleDeepika Kanyan, Miriana Horacek-Glading, Martijn J Wildervanck, Tilo Söhnel, David C Ware, Penelope Jane Brothers
      Sugar-O-BODIPY conjugates, in which the fluorescent dye O-BODIPY is linked to sugars directly through B-O-C bonds, have been synthesized via an acid-catalyzed transesterification procedure. Conjugates of glucose, xylose and ribose...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • The Application of C-H bond Functionalization in Total Syntheses of Indole
           Natural Products

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01636A, Review ArticleDong-Xing Tan, Fu-She Han
      The direct functionalization of unactivated C–H bonds is a rapidly growing field in organic chemistry in recent years because of its indisputable advantages in bond forming reactions in terms of...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Head-to-tail cyclization for synthesis of naturally occurring cyclic
           peptides on organophosphous small-molecular supports

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01362A, Research ArticleHaidi Li, Junyou Li, Jie Chao, Zixin Zhang, Chuanguang Qin
      To achieve the head-to-tail cyclic peptides via the liquid-phase on-support cyclization and synergistic self-cleavage strategy, 4,4’-bis(diphenylphosphinyloxyl) diphenyl ketoxime (BDKO) and 4-diphenyl phospholoxy benzyl alcohol (DPBA) were designed and prepared as...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Palladium-catalyzed tandem hydrocarbonylative cycloaddition for expedite
           construction of bridged lactones

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01568K, Research ArticleHanmin Huang, Yongzheng Ding, Min Si
      A palladium-catalyzed tandem carbonylative lactonization and cycloaddition reaction of 2-vinyl acetophenones with alkenes and CO has been established. This reaction enables an efficient conversion of the easily available alkenes to...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • From α-Keto Acids to Nitrile Oxides Enabled by Copper Nitrate: A Facile
           Access to Fused Isoxazolines

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01574E, Research ArticleYuping Zhu, Tianqi Liu, Bingxin Liu, Houguang Shi, Qitao Tan, Bin Xu
      α-Keto acids were unprecedentedly employed as novel precursors of nitrile oxides on treatment with copper nitrate, which reacted with maleimides via [3+2] dipolar cycloaddition leading to pharmacologically interesting fused isoxazolines....
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Tunable Photocatalytic Oxysulfonylation and Chlorosulfonylation of α-CF3
           Alkenes with Sulfonyl Chlorides

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01686E, Research ArticlePeng-Ju Xia, Fu Liu, Shu-Hui Li, Jun-An Xiao
      Tunable photoredox-catalyzed chlorosulfonylation and oxysulfonylation of α-trifluoromethylstyrenes with sulfonyl chloride were facilely achieved by simply manipulating photocatalyst and solvent. This strategy makes full use of the structural features of sulfonyl...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Recent advances in asymmetric reduction of imines by recycled catalyst
           systems

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01526E, Review ArticleLidan Deng, Xingwang Liu, Shihua Song
      Chiral amines are widely found in nature, many of which possess significant biological and synthetic values. The catalytic asymmetric syntheses of optically active amines have inspired enormous interests. Currently, the...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Planar Blatter radicals through Bu3SnH and TMS3SiH–assisted cy-clization
           of aryl iodides: Azaphilic radical addition

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01742J, Research ArticlePiotr Kaszynski, Paulina Bartos, Małgorzata Celeda, Anna Pietrzak
      Bu3SnH and TMS3SiH–assisted cyclizations of iodoarene derivatives of the benzo[e][1,2,4]triazine lead to the formation of planar Blatter radicals (2-phenyl-3H-[1,2,4]triazino[5,6,1-kl]phenoxazin-3-yls and 2-phenyl-3H-[1,2,4]triazino[5,6,1-kl]phenothiazin-3-yls) in yields up to 96%. The cyclization step involves...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Asymmetric catalytic nitrooxylation and azidation of β-keto amides/esters
           with hypervalent iodine reagents

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01634B, Research ArticleChangqiang He, Zhikun Wu, Yuqiao Zhou, Weidi Cao, Xiaoming Feng
      Chiral Lewis acid-catalyzed enantioselective nitrooxylation of cyclic and acyclic β-keto amides/esters with hypervalent iodine(III) reagents is reported. A number of α-nitrooxy-β-keto amides/esters were obtained with good yields and high enantioselectivities...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Direct Synthesis β-Acyloxy Aldehydes from Linear Allylic Esters Using
           O2 as Sole Oxidant

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01607E, Research ArticleShu-Hui Lei, Ya Zhong, Xian-Peng Cai, Qing Huang, Jian-Ping Qu, Yan-Biao Kang
      A simple and practical preparation of β-O substituted aldehydes directly from linear allylic esters is developed. Using bis(benzonitrile)palladium chloride as the catalyst and O2 as sole oxidant, the tandem isomerization-...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Decarbonylative Sonogashira cross-coupling: a fruitful marriage of alkynes
           with carboxylic acid electrophiles

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      Abstract: Org. Chem. Front., 2022, Advance Article

      DOI : 10.1039/D1QO01539G, HighlightChengwei Liu, Michal Szostak
      The Sonogashira cross-coupling is one of the most fundamental C–C bond-forming reactions, wherein the strategic value of an alkyne moiety has found widespread applications at the frontiers of organic chemistry, materials science and drug discovery as the cornerstone building block of chemical synthesis.
      To cite this article before page numbers are assigned, use the
      DOI form of citation above.
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Photochemical and electrochemical strategies in C-F bonds activation and
           functionalization

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01512E, Review ArticleZhanghong Wang, Yu Sun, Liu-Yu Shen, Wen-Chao Yang, Fei Meng, Pinhua Li
      The activation and functionalization of C-F bonds under mild conditions can serve as an important tool for organic syntheses including the modification of pharmaceuticals or agrochemicals and the synthesis of...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Mechanistic Insights into Nickel- and Gold-Catalyzed Diastereoselective [4
           

    • Free pre-print version: Loading...

      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01468D, Research ArticleKang Lv, Xiaoguang Bao
      Density functional theory (DFT) calculations were performed to gain an in-depth mechanistic understanding on the Ni(0)- and Au(I)-catalyzed diastereoselective [4 + 2 + 1] cycloadditions between dienynes and diazo compounds....
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Eugenunilones A-H: Rearranged Sesquiterpenoids from Eugenia uniflora

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01629F, Research ArticleMu Chen, Jia-Qing Cao, Song Ang, Ting-Ni Zeng, Ni-Ping Li, Tang-Jia Yang, Jun-Shan Liu, Yan Wu, Wen-Cai Ye, Lei Wang
      Six rearranged sesquiterpenoid dimers and monomers with four kinds of new skeletons, meso-eugenunilone A (meso-1), (+)- and (-)-eugenunilones B-F [(+)-and (-)-2-6], along with two new biogenetically related members (+)- and...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
  • Metal-free Synthesis of N-Sulfonylformamidines via Skeletal Reconstruction
           of Sulfonyl Oximonitriles

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      Abstract: Org. Chem. Front., 2022, Accepted Manuscript

      DOI : 10.1039/D1QO01665B, Research ArticleFeng Li, Ziyan Wu, Jingjing Wang, Siyuan Zhang, Jiaxin Yu, Zhen Yuan, Jingya Liu, Renzeng Shen, Yao Zhou, Lantao Liu
      We firstly develop an unprecedented domino reaction of sulfonyl oximonitriles with secondary amines to streamline synthesis of N-sulfonylformamidines in decent to high yields under mild reaction conditions. In addition, the...
      The content of this RSS Feed (c) The Royal Society of Chemistry
       
 
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